Near-field probing of image phonon-polaritons in hexagonal boron nitride on gold crystals

Sergey G. Menabde, Sergejs Boroviks, Jongtae Ahn, Jacob T. Heiden, Kenji Watanabe, Takashi Taniguchi, Tony Low, Do Kyung Hwang, N. Asger Mortensen*, Min Seok Jang

*Corresponding author for this work

Research output: Contribution to journalJournal articleResearchpeer-review

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Abstract

Near-field mapping has been widely used to study hyperbolic phonon-polaritons in van der Waals crystals. However, an accurate measurement of the polaritonic loss remains challenging because of the inherent complexity of the near-field signal and the substrate-mediated loss. Here we demonstrate that large-area monocrystalline gold flakes, an atomically flat low-loss substrate for image polaritons, provide a platform for precise near-field measurement of the complex propagation constant of polaritons in van der Waals crystals. As a topical example, we measure propagation loss of the image phonon-polaritons in hexagonal boron nitride, revealing that their normalized propagation length exhibits a parabolic spectral dependency. Furthermore, we show that image phonon-polaritons exhibit up to a twice longer normalized propagation length, while being 2.4 times more compressed compared to the case of the dielectric substrate. We conclude that the monocrystalline gold flakes provide a unique nanophotonic platform for probing and exploitation of the image modes in low-dimensional materials.

Original languageEnglish
Article numbereabn0627
JournalScience Advances
Volume8
Issue number28
ISSN2375-2548
DOIs
Publication statusPublished - Jul 2022

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