Extremely confined gap plasmon modes: when nonlocality matters

Sergejs Boroviks, Zhan Hong Lin, Vladimir A. Zenin, Mario Ziegler, Andrea Dellith, P. A.D. Gonçalves, Christian Wolff, Sergey I. Bozhevolnyi, Jer Shing Huang, N. Asger Mortensen*

*Corresponding author for this work

Research output: Contribution to journalJournal articleResearchpeer-review

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Abstract

Historically, the field of plasmonics has been relying on the framework of classical electrodynamics, with the local-response approximation of material response being applied even when dealing with nanoscale metallic structures. However, when the confinement of electromagnetic radiation approaches atomic scales, mesoscopic effects are anticipated to become observable, e.g., those associated with the nonlocal electrodynamic surface response of the electron gas. Here, we investigate nonlocal effects in propagating gap surface plasmon modes in ultrathin metal–dielectric–metal planar waveguides, exploiting monocrystalline gold flakes separated by atomic-layer-deposited aluminum oxide. We use scanning near-field optical microscopy to directly access the near-field of such confined gap plasmon modes and measure their dispersion relation via their complex-valued propagation constants. We compare our experimental findings with the predictions of the generalized nonlocal optical response theory to unveil signatures of nonlocal damping, which becomes appreciable for few-nanometer-sized dielectric gaps.

Original languageEnglish
Article number3105
JournalNature Communications
Volume13
Issue number1
Number of pages8
ISSN2041-1723
DOIs
Publication statusPublished - Jun 2022

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