Surface Modification Enabling Reproducible Cantilever Functionalization for Industrial Gas Sensors

Daniel Mamou, Lawrence Nsubuga, Tatiana Lisboa Marcondes, Simon Overgaard Høegh, Jeanette Hvam, Florian Niekiel, Fabian Lofink, Horst-Günter Rubahn, Roana de Oliveira Hansen*

*Kontaktforfatter

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Abstract

Micro-cantilever sensors are a known reliable tool for gas sensing in industrial applications. We have demonstrated the application of cantilever sensors on the detection of a meat freshness volatile biomarker (cadaverine), for determination of meat and fish precise expiration dates. For achieving correct target selectivity, the cantilevers need to be functionalized with a cadaverineselective
binder, based on a cyclam-derivative. Cantilever surface properties such as surface energy strongly influence the binder morphology and material clustering and, therefore, target binding. In this paper, we explore how chemical and physical surface treatments influence cantilever surface, binder morphology/clustering and binding capabilities. Sensor measurements with non-controlled surface properties are presented, followed by investigations on the binder morphology versus surface energy and cadaverine capture. We demonstrated a method for hindering binder crystallization on functionalized surfaces, leading to reproducible target capture. The results show that cantilever surface treatment is a promising method for achieving a high degree of functionalization reproducibility for industrial cantilever sensors, by controlling binder morphology and uniformity.
OriginalsprogEngelsk
Artikelnummer6041
TidsskriftSensors
Vol/bind21
Udgave nummer18
Antal sider8
ISSN1424-8220
DOI
StatusUdgivet - 9. sep. 2021

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